A Stretchable Expanded Polytetrafluorethylene-Silicone Elastomer Composite Electret for Wearable Sensor

Soaring developments in wearable electronics raise an urgent need for stretchable electrets. However, achieving soft electrets simultaneously possessing excellent stretchability, longevity, and high charge density is still challenging. Herein, a facile approach is proposed to prepare an all-polymer hybrid composite electret based on the coupling of elastomer and ePTFE membrane. The composite electrets are fabricated via a facile casting and thermal curing process. The obtained soft composite electrets exhibit constantly high surface potential (−0.38 kV) over a long time (30 days), large strain (450%), low hysteresis, and excellent durability (15,000 cycles). To demonstrate the applications, the stretchable electret is utilized to assemble a self-powered flexible sensor based on the electrostatic induction effect for the monitoring of human activities. Additionally, output signals in the pressure mode almost two orders of magnitude larger than those in the strain mode are observed and the sensing mechanism in each mode is investigated.