Nyimboyi debuted panguva nhamba mbiri musi Irish Singles Chart musi 19 November 2013, zuva pashure rakanga rabudiswa; yaiva imwe nhatu One Direction nziyo pamusoro 10 kuti vhiki, pamwe Album wacho musoro njanji "Midnight Memories" (nhamba nhatu) uye "Nhau My Life" (nhamba nhanhatu). One Direction yakaita rwiyo rwacho pane zvose zviviri zvemafambiro avo makuru emakwikwi: Kwatiri Tiri Tour
(2014) uye On the Road Again Tour (2015).